Lanthanide oxide/zirconium oxide atomic layer deposited...

Active solid-state devices (e.g. – transistors – solid-state diode – Field effect device – Having insulated electrode

Reexamination Certificate

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C257S310000

Reexamination Certificate

active

06989573

ABSTRACT:
The invention provides a laminated dielectric layer for semiconductor devices formed by a combination of ZrO2and a lanthanide oxide on a semiconductor substrate and methods of making the same. In certain methods, the ZrO2is deposited by multiple cycles of reaction sequence atomic layer deposition (RS-ALD) that includes depositing a ZrI4precursor onto the surface of the substrate in a first pulse followed by exposure to H2O/H2O2in a second pulse, thereby forming a thin ZrO2layer on the surface. After depositing the ZrO2layer, the lanthanide oxide layer is deposited by electron beam evaporation. The composite laminate zirconium oxide/lanthanide oxide dielectric layer has a relatively high dielectric constant and can be formed in layers of nanometer dimensions. It is useful for a variety of semiconductor applications, particularly for DRAM gate dielectric layers and DRAM capacitors.

REFERENCES:
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patent: 2004/0219746 (2004-11-01), Vaartstra et al.
patent: 2005/0077519 (2005-04-01), Ahn et al.
Jeon, Sanghun, et al., “Excellent Electrical Characteristics of Lanthanide Oxide and Lanthanide-doped Oxide for MOS Gate Dielectric Applications,” IEEE, 2001, pp. 01-471 to474.
Kukli, Kaupo, et al., “Influence of thickness and growth temperature one the properties of zirconium oxide films grown by atomic layer deposition on silicon,” Thin Solid Films 410, 2002, pp. 53-60.
Kukli, Kaupo, et al., “Dielectric Properties of Zirconium Oxide Grown by Atomic Layer Deposition from Iodide Precursor,” Journal of The Electrochemical Society, vol. 148, No. 12, 2001.
Kukli, Kaupo, et al., “Properties of Ta2O5-Based Dielectric Nanolaminates Deposited by Atomic Layer Epitaxy,” Journal of The Electrochemical Society, vol. 144, No. 1, 1997, pp. 300-306. Jan. 1997.
Kukli, Kaupo, et al., “Atomic layer deposition of zirconium oxide from zirconium tetraiodide, water and hydrogen peroxide,” Journal of Crystal Growth, vol. 231, 2001, pp. 262-272.
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