Hexakis(monohydrocarbylamino)disilanes and method for the...

Semiconductor device manufacturing: process – Coating of substrate containing semiconductor region or of... – By reaction with substrate

Reexamination Certificate

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C438S791000, C438S786000, C438S778000

Reexamination Certificate

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07064083

ABSTRACT:
A composition and method of preparation, to provide silane compounds that are free of chlorine. The compounds are hexakis(monohydrocarbylamino)disilanes with general formula (I)in-line-formulae description="In-line Formulae" end="lead"?((R)HN)3—Si—Si—(NH(R))3  (I)in-line-formulae description="In-line Formulae" end="tail"?wherein each R independently represents a C1to C4hydrocarbyl. These disilanes may be synthesized by reacting hexachlorodisilane in organic solvent with at least 6-fold moles of the monohydrocarbylamine RNH2(wherein R is a C1to C4hydrocarbyl). Such compounds have excellent film-forming characteristics at low temperatures. These films, particularly in the case of silicon nitride and silicon oxynitride, also have excellent handling characteristics.

REFERENCES:
International Search Report for PCT/EP02/13790.
Chemical Abstracts Service; Schuh, Heinz et al: “Disilanylamines. Compounds comprising the structural unit silicon-silicon-nitrogen, as single-source precursors for plasma-enhanced chemical vapor deposition (PE-CVD) of silicon nitride”.
Chemical Abstracts Service; Wrackmeyer, Bernd et al: “Carbon-13, nitrogen-15 and silicon-29 nuclear magnetic resonance studies of some aminosilanes and aminodisilanes”.

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