Bleaching of lignocellulosic material with in-situ-generated dio

Paper making and fiber liberation – Processes of chemical liberation – recovery or purification... – Treatment with particular chemical

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162 76, 162 78, 162 82, D21C 320, D21C 916

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053665937

ABSTRACT:
A chemical pulp which contains reactants capable of generating dioxirane within the pulp is produced in a process which comprises mixing a pulp with reactants comprising a carbonyl compound, preferably acetone, and an oxygen donor, preferably monoperoxysulfate, in proportions which produce a water-soluble dioxirane having a molecular diameter of less than 140 angstrom units. Such a pulp bleaching process which employs dioxirane as a bleaching agent is rendered environmentally and economically acceptable by recycling the reactants employed to produce the dioxirane.

REFERENCES:
patent: 3822114 (1974-07-01), Montgomery
patent: 4404061 (1983-09-01), Cael
Adam et al., "Dioxirane Epoxidation of alpha, beta-Unsaturated Ketones", Chem. Ber. 124 (1991), 227-232.
Edwards et al., "On the Formation and Reactivity of Dioxirane Intermediates in the Reaction of Peroxoanions with Organic Substrates," Photochem. and Photobiol., vol. 10, pp. 63-70 (1979).
Zabrowski et al., "The Oxidation of Aromatic Amines in the Presence of `Electron-Rich` Aromatic Systems," Tetrahedron Letters, vol. 29, No. 36, pp. 4501-4504 (1988).
SINGH, "The Bleaching of Pulp", Tappi Press, Atlanta, Ga. 1979, pp. 305-314.
Montgomery, "Catalysis of Peroxymonosulfate Reactions by Ketones," J. Amer. Soc., vol. 96, No. 25, pp. 7820, 7821 (1974).
Murray et al., "Dioxiranes: Synthesis and Reactions of Methyldioxiranes," J. Org. Chem. 1985, 50, 1847-2853.

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