T-butoxycarbonylaminoethylamine for the synthesis of PNA...

Organic compounds -- part of the class 532-570 series – Organic compounds – Carboxylic acid esters

Reexamination Certificate

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C560S155000

Reexamination Certificate

active

06919476

ABSTRACT:
A process for amino acid derivatives shown by the below general formula (I):(wherein R1means a hydrogen atom or a straight chain or branched chain alkyl group with 1-5 carbon atoms.) having an object to provide a process of the amino acid derivatives of the formula (I) and their synthetic intermediate, t-butoxycarbonylamino-ethylamine, whereby it requires no tedious procedure and is also good in yield, and its application to a mass production is easy, and to provide novel amino acid derivatives of the formula (IV), their synthetic intermediates, and a process thereof, characterized in that it comprises a step to obtain the amino acid derivatives shown by the general formula (I) by hydrolysis of compounds shown by the below formula (II):(wherein R1has the same meaning as described above, and R2means a straight chain or branched chain alkyl group with 1-4 carbon atoms.) as well as amino acid derivatives shown by the general formula (IV):(wherein R1means a hydrogen atom or a straight chain or branched chain alkyl group with 1-5 carbon atoms, and n means any one of integers 1-11.), and a process for the amino acid derivative, characterized in that it comprises a reduction step of benzyloxycarbonyl-ω-amino acid derivatives.

REFERENCES:
patent: 5595741 (1997-01-01), Huber et al.
patent: WO 97/30053 (1997-08-01), None
patent: WO 99/31121 (1999-06-01), None
patent: WO 2002020470 (2002-03-01), None
patent: WO 2002051797 (2002-07-01), None
Roeske et al, Journal of Organic Chemistry, vol. 41(7), (1976), pp1260-1261.
Roeske, Roger W., Selective Reduction of the Amide Carbonyl Group in Depeptides by Borane, J. Org. Chem. vol. 41, No. 7, 1976, pp 1260-1261.

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