Process for the preparation of macrocyclic chelants and the chel

Organic compounds -- part of the class 532-570 series – Organic compounds – Unsubstituted hydrocarbyl chain between the ring and the -c-...

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540465, 424 9363, C07F 96524, C07D29518

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active

059257520

ABSTRACT:
A process for the preparation of complexes of macrocyclic chelants with paramagnetic metal trivalent ions of formula (XII) ##STR1## wherein R.sub.1, R.sub.2 and Me.sup.3+ are as described in the following, comprising: a) reaction of 1,4,7,10-tetraazacyclododecane with triethyl orthoformate to give carboxymethylation reaction in water; c) hydrolysis reaction in basic conditions; d) alkylation according to known methods with an epoxide in water; e) complexation according to known methods carried out in water by addition of a paramagnetic metal salt; f) purification by diafiltration, final desalting of the aqueous solution on ion exchange resins and g) crystallization or recovery.

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patent: 5447635 (1995-09-01), Viscardi et al.
patent: 5747000 (1998-05-01), Platzek et al.
Dischino et al., Inorg. Chem. 1991, 30, pp. 1265-1269.
Weisman et al., Tetrahedram Letters., vol. 21, 1980 pp. 3635-3638.

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