Ionic modification of organic resins and photoresists to produce

Radiation imagery chemistry: process – composition – or product th – Imaging affecting physical property of radiation sensitive... – Radiation sensitive composition or product or process of making

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430191, 430270, 430914, 430925, G03F 709

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active

053936426

ABSTRACT:
A photoresist composition is disclosed that comprises an organic resin that is thermoset by acid catalysis and a photoactive, etch-resistant ionic modifier formed of an anion and a cation. The modifier is present in the organic resin in an amount effective to produce substantial photoreactivity and etch resistance in a mixture of the resin and the modifier. The cation will, upon exposure to electromagnetic radiation, produce a species that is weakly basic or neutral, and the anion will, upon exposure to electromagnetic radiation, produce an acid precursor that will form a relatively strong acid in an acid-base solvent system. As a result, the relatively strong acid will catalyze the organic resin upon exposure to an appropriate frequency of electromagnetic radiation and the relatively weak base or neutral species formed by the cation will not substantially neutralize the acid or interfere with the acid catalyzed reaction of the organic resin.

REFERENCES:
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patent: 5114827 (1992-05-01), Tranjan et al.
"Photolysis of Tris (4-tert-butoxycarbonyloxyphenyl) Sulphonium Salts. A Mechanistic Study," Reinhold Schwalm, Ruth Bug, Guang-Song Dai, Peter M. Fritz, Michael Reinhardt, Siegfried Schneider and Wolfram Schnabel, J. Chem. Soc. Perkin Trans. 2, 1991.
"Electrochemical Degradation of Aryl Sulfonium Salts," Manuel Finkelstein, Raymond C. Peterson, and Sidney D. Ross, Journal of the Electrochemical Society, vol. 110, No. 5, May 1963.
"A New Mechanism for Photodecomposition and Acid Formation from Triphenylsulphonium Salts," John L. Dektar and Nigel P. Hacker, J. Chem. Soc., Chem. Commun., 1987.
"Photochemistry of Aromatic Ions. Photolysis of Quaternary Anilinium Salts," Thomas D. Walsh, Robert C. Long, Journal of the American Chemical Society, 89, 3943 (1967).
"Photolysis of Benzyltriphenylphosphonium and Tetraphenylphosphonium Chlorides," C. E. Griffin and M. L. Kaufman, Tetrahedron Letters No. 12, pp. 773-775, 1965. Pergamon Press Ltd.
"The Electroreduction of Quaternary Ammonium Compounds," Jaspal S. Mayell and Allen J. Bard, Electroreduction of Quaternary Ammonium Compounds, Feb. 20, 1963.

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