Hydroformylation process employing rhodium-based catalysts compr

Organic compounds -- part of the class 532-570 series – Organic compounds – Oxygen containing

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252431P, 568909, 568455, C07C 4510

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042217440

ABSTRACT:
An improved process for hydroformylating an ethylenically-unsaturated compound to form an aldehyde derivative thereof in the presence of rhodium hydridocarbonyl in complex combination with an organic ligand, characterized by employing as said organic ligand a compound having two phosphino moieties, one being of the formula: ##STR1## and the other being of the formula: ##STR2## wherein R.sub.1, R.sub.2, R.sub.1 ', and R.sub.2 ' are organic radicals at least one of which contains an electronegative substituent moiety. The presence of the electronegative substituent in the ligand leads to an increased ratio of linear aldehyde to branched-chain aldehyde in the hydroformylation reaction product.

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Marchuk et al., "Chem. Abst.", vol. 66, p. 7609v.

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