Preparation of ionomers and polyurethane elastomers from carboxy

Synthetic resins or natural rubbers -- part of the class 520 ser – Synthetic resins – From reactant having at least one -n=c=x group as well as...

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528 50, 528 75, 528 81, 528 83, 556114, 556131, 556136, 556147, 560198, C08G 1846, C08G 1850, C07C 6708, C07F 310, C07F 1500

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045902550

ABSTRACT:
A process for making metal salt (ionomers) of carboxylic acid-containing mono- and polyether polyol addition products by (1) reacting maleic acid, fumaric acid, itaconic acid, or mixtures thereof with at least one polyhydroxy-containing mono- or polyether compound (e.g. a polyether diol or triol) in the presence of a peroxy-type free radical initiator to form a carboxylic acid group-containing addition product and (2) neutralizing said addition product with a sufficient amount of metal ions selected from the group consisting of metals from Groups 1a, 2a, 8, 1b and 2b of the Periodic Table to convert at least about 10% of the carboxylic acid groups to ionomeric salt groups. These ionomers may be then changed into useful polyurethane elastomers by reaction with organic polyisocyanates.

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D. Dieterich; Polyurethane Ionomers, a New Class of Block Polymers, Angew. Chem. Internat. Edit., vol. 9 (1970), No. 1, pp. 40-50.
V. Malatesta and J. C. Scaiano, "Absolute Rate Constants for the Reactions of tert-Butoxyl with Ethers: Importance of the Stereoelectronic Effect", J. Org. Chem., 1982, 47, pp. 1455-1459.

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