Variable pressure ionization detector for gas chromatography

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250382, G01N 2770

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active

047218584

ABSTRACT:
Method and apparatus for differentiating organic compounds based on their electron affinity. An electron capture detector cell (ECD) is operated at pressures ranging from atmospheric to less than 1 torr. Through variation of the pressure within the ECD cell, the organic compounds are induced to either capture or emit electrons. Differentiation of isomeric compounds can be obtianed when, at a given pressure, one isomer is in the emission mode and the other is in the capture mode. Output of the ECD is recorded by chromatogram. The invention also includes a method for obtaining the zero-crossing pressure of a compound, defined as the pressure at which the competing emission and capture reactions are balanced and which may be correlated to the electron affinity of a compound.

REFERENCES:
patent: 3601609 (1971-08-01), Yauger, Jr.
patent: 4137453 (1979-01-01), Siegel
patent: 4166379 (1979-09-01), Bradshaw
Michelle V. Buchanan and Geraldine Olerich, "Differentiation of Polycyclic Aromatic Hydrocarbons Using Electron Capture Negative Chemical Ionization", Organic Mass Spectrometry, vol. 19, No. 10, (1984), pp. 486-489.
Littlewood, A. B., "Electron Capture Detector" In: Gas Chromatography: Principles, Techniques, and Applications (New York, Academic Press, 1970), pp. 315-322.

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