Supported heteropoly acid catalysts for isoparaffin-olefin alkyl

Chemistry of hydrocarbon compounds – Saturated compound synthesis – By condensation of a paraffin molecule with an olefin-acting...

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585722, 585725, 585732, C07C 258

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053248813

ABSTRACT:
The alkylation of isoparaffin with olefin to provide alkylate is carried out in the presence of, as catalyst, a supported heteropoly acid. The support may be MCM-41, and the heteropoly acid may be dodecawolframophosphoric acid (i.e., phosphotungstic acid, i.e., H.sub.3 PW.sub.12 O.sub.40).

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Nowinska, K. et al., "Catalytic Activity of Supported Heteropoly Acids for Reactions requiring Strong Acid Centres," J. Chem. Soc., 87(5), 749-753 (1991).
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Ono, Y. et al., "The Catalytic Behavior of Metal Salts of Heteropolyacids in the Vapor-phase Synthesis of Methyl t-Butyl Ether," Tokyo Institute of Tech (1984) pp. 405-416.
Matsuda, T. et al., "Effect of Pretreatment of the Acidity of Heteropoly Compounds in Butene Isomerization," J. Chem. Soc., 77, 3107-3117 (1981).
Nowinska, K. "Evidence for Superacid Sites on the Ammonium Salt of 12-Tungstophosphoric Acid from a Catalytic Test Reaction," J. Chem. Soc., 44 (1990).

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