Solution polymerization

Synthetic resins or natural rubbers -- part of the class 520 ser – Synthetic resins – Polymers from only ethylenic monomers or processes of...

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C08F 452

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active

043025684

ABSTRACT:
A composition useful as a catalyst in solution polymerization comprises (1) a barium, calcium and/or strontium alcoholate, (2) an organoaluminum compound and (3) an organomagnesium compound. (2) and (3) may be used as a complex with (1). The compositions can be used to polymerize ethylenically unsaturated monomers like butadiene, butadiene and styrene, and isoprene and heterocyclic monomers like oxiranes, thiiranes, siloxanes, thiatanes and lactams. The catalyst composition can produce polybutadienes and butadiene-styrene copolymers having a trans-1,4 content as high as 90%. The non-terminating features of the polymerization of this invention permit the preparation of functionally terminated butadiene based polymers and block polymers containing sufficient amounts of trans-1,4 butadiene units to crystallize.

REFERENCES:
patent: 3448092 (1969-06-01), Chiang
patent: 3526604 (1970-09-01), Wadsworth
patent: 3578642 (1971-05-01), Mueller et al.
patent: 3631006 (1971-12-01), Hawkins
patent: 3687916 (1972-08-01), Mueller et al.
patent: 3846385 (1974-11-01), Hargis et al.
patent: 4080492 (1978-03-01), de Zarauz
patent: 4112210 (1978-09-01), de Zarauz
Physico-Chemical Res. Insti., Polymer Science, USSR, 18(9), 2325-2329, (1976).
Lithium Corp. of America, "Product Bulletin" on "Dibutyl Magnesium", (P-430), 4-78.
Rubber Chemistry and Technology, vol. 42, No. 4, Sep. 1969, pp. 1040-1053.

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