Regioselective production of para-dialkyl benzenes

Chemistry of hydrocarbon compounds – Aromatic compound synthesis – By alkyl or aryl transfer between molecules – e.g.,...

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585467, C07C 552

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active

054751799

ABSTRACT:
A method for the selective disproportionation of a substituted aromatic compound wherein the aromatic compound is passed over a catalytic molecular sieve which has been pre-selectivated with a silicon deposit and then subsequently treated with a silicon-containing, high efficiency p-xylene selectivating agent at conversion conditions. The present invention attains para-xylene product over 95% at a toluene conversion of at least 20%. The present invention also includes the highly para-selective catalyst which results from the pre-selectivation and subsequent treatment of a catalytic molecular sieve with a high efficiency p-xylene selectivating agent under the recited conditions.

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Hibino, et al., "Shape Selectivity Over HZSM-5 Modified by Chemical Vapor Deposition of Silicone Alkoxide," Journal of Catalysis, 12, 551-558 (1991).

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