Regeneration of spent hydrodesulfurization catalyst with heterop

Compositions – Preservative agents – Anti-oxidants or chemical change inhibitants

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208216R, 252412, 252414, 423 68, 423150, B01J 2394, B01J 2392, B01J 2120, C10G 2302

Patent

active

042724015

ABSTRACT:
Contacting deactivated hydrodesulfurization catalyst, such as Co-Mo supported on alumina, with a heteropoly acid, such as molybdophosphoric acid or tungstosilicic acid, in pH range of about 1 to 3 and temperature range of about 20.degree. to 80.degree. C., results, before any coke is burned off the catalyst, in selective abstraction of vanadium and nickel, removal of sulfur, increase in surface area, and increase in pore volume of the catalyst. Subsequent cobalt doping of demetallized catalyst followed by calcination promotes decoking, additional sulfur removal and additional increase in surface area and pore volume. The process results in substantially complete regeneration of catalytic activity.

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