Quality control system for monitoring and control of...

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Reexamination Certificate

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C209S011000, C209S913000, C034S132000, C034S179000

Reexamination Certificate

active

06533124

ABSTRACT:

FIELD OF THE INVENTION
This invention relates to a quality control (QC) system for continuous sampling and monitoring of contaminants in recycled plastic materials. More specifically, the present invention relates to a QC system for sampling and determining the presence of certain substances, such as contaminants, within plastic material recycled from polyethylene terepthalate (PET) containers. In further aspect, the QC system herein also uniquely provides for direct in-plant continuous control and detection of contaminants in post-consumer recycled plastic materials thereby expanding post-consumer recycled plastic material markets and applications.
BACKGROUND OF THE INVENTION
Plastic material is now common in everyday life, and ultimately, when used as a disposable product, plastic has also found itself as a significant contributor to the problem of solid waste management. With respect to solid waste management, several different options have been identified to date to deal with the ever increasing need to conserve the valuable and non-renewal resources associated with plastic material production and disposal. For example, “source reduction” which refers to a reduction in the amount of material that is used in any application, and, therefore, a reduction in the amount of material potentially discarded when that use is completed.
However, recycling remains a much more environmentally favored route over “source reduction”, and is based upon the reprocessing and refabrication of a plastic material that has been used and discarded by the consumer which otherwise would be destined for disposal. This type of recycling has now become well known as post-consumer recycling (PCR), as opposed to recycling that develops as part of the reuse of by-products from a plastic manufacturing process (which by-products are generally known as “regrind”).
Unfortunately, the reprocessing and refabrication of PCR materials into useful products requires several steps (collection, handling/sorting, reclamation/cleaning and end-use fabrication) and presents unique problems. That is, each of these steps has remained relatively expensive, not the least of which is the requirement to insure that the recycled plastic material at issue is clean and safe for consumer reuse. In that regard, it is an altogether simple matter to envision that while in the hands of consumers, intentionally or otherwise, plastic materials can and will come into contact with other more toxic chemicals, and as plastic materials can absorb such toxins, this requires cleaning and detection (of any residual toxins) prior to placement of such material back into the consumer's hands. Of course, this is even more the case to the extent that the recycled material is targeted for an application involving direct food or beverage contact.
Not surprisingly therefore, and to assure consumer safety, regulatory agencies promptly became active with respect to the use of PCR material for food/beverage applications. For example, in 1992 the Food and Drug Administration published proposed guidelines for recycling, which divided plastics recycling into three classes: Primary recycling of plastics which are plant scrap without any consumer exposure; Secondary recycling involving the physical cleaning of post-consumer plastics by physical processes such as washing, vacuum and heat treatment; and Tertiary recycling involving chemical treatment, usually depolymerization (breaking the plastic material down into its building blocks, known as “monomers”), followed by monomer purification and reconstitution back to plastic material. See, “Points to Consider for the Use of Recycled Plastics in Food Packaging: Chemistry Considerations”, U.S. FDA, Center for Food Safety and Applied Nutrition (HFS-245), Washington, D.C. April 1992.
With regards to secondary recycling, it should now be apparent that central to any efficient physical cleaning operation is the need to monitor the washing procedures to determine whether or not any recycled plastic material at issue is void of residual contaminant, or whether or not the residual contaminant is present at a level such that it would not migrate out when placed in contact with a food/beverage media. For further discussion see, e.g., “
The Threshold of Regulation and its Application to Indirect Food Additive Contaminants in Recycled Plastics
”, Food Additives and Contaminants”, 1997, Vol. 14, No. 6-7, 661-670.
Toward such monitoring objectives, a variety of U.S. Patents have been issued directed at sampling and determining the presence of contaminants in recyclable plastic materials, which for the most part have been based upon the well-known analytical tool known as gas chromatographic (GC) instrumentation. Chromatography provides timewise separation of gases or liquid samples as part of analyses in which specific compounds are detected. This timewise separation achieved among constituents permits particular compounds to be distinguished from interferents and from other specific compounds of interest by signal peaks which occur at distinct times at the output of detectors downstream of the chromatograph. The times at which the detector “detects” a given constituent, as well as the amplitude and shape can be predetermined by calibration techniques using samples of known composition, and detection systems containing the chromatographs can be electronically programmed to provide alarms or specific responses upon detection of each compound of interest.
For example, in U.S. Pat. No. 5,073,203, entitled “Method for Recycling Polyethylene Terephthalate (PET) Beverage Bottles by Treating with Carbon Dioxide”, there is disclosed a method for recycling polymer materials based on PET used for food packaging such as beverage bottles. As disclosed therein, when such PET resin, in the form of crushed bottles, is washed/extracted by a fluid such as supercritical CO
2
, at preferred temperatures between 31° and 245° C., the contaminants therein are removed, without any effect on the PET intrinsic viscosity. The washed PET is then tested by GC equipment, and the GC tests therein indicated that under such conditions the contaminant material had been successfully removed.
Attention is also directed to U.S. Pat. Nos. 4,830,192, 4,858,768 and 5,067,616 which describes a method of discriminating between contaminated and uncontaminated containers prior to washing by testing the residue of the container to determine if the residue is the residue of the original product in the container. If the residue is not sufficiently similar to the original product, the container is rejected as contaminated.
Other related disclosures of interest include U.S. Pat. No. 5,108,705, which discloses a method and apparatus for high speed, selective detection of vapors of specific compounds, utilizing a bypass branch and high speed gas chromatography for improved selectivity and detection. In U.S. Pat. No. 4,843,016 a detection system is disclosed for detecting the presence of predetermined compounds in a sample. This system similarly comprises a sample injector, a chromatographic column, a conversion means and one or more specific gas detectors. The conversion means is said to transform the column effluent to combustion products in the gas phase, after which those combustion products are transferred to the specific gas detectors.
In U.S. Pat. No. 4,880,120, entitled “Plastic Container Inspection Process”, there is disclosed a container inspection process for detecting the presence of contaminants in plastic containers. More specifically, the process flushes volatiles from within the container by injecting gas, draws a vapor sample from within the container and analyzes the sample by ionization techniques.
In U.S. Pat. No. 5,352,611 there is disclosed a method and apparatus for samples and determining the presence of residues of contaminants in containers. The method includes the steps of injecting a fluid described as air or CO
2
into the containers in order to displace a portion of the contents, evacuating a sample of the container contents so displaced by

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