Process for the synthesis and purification of diisopropenylbenze

Chemistry of hydrocarbon compounds – Aromatic compound synthesis – Having alkenyl moiety – e.g. – styrene – etc.

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585254, 585277, 585315, 585321, C07C 5333

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active

045284130

ABSTRACT:
Diisopropenylbenzene is a monomer that can be used in the preparation of many useful polymers and is also a chemical intermediate that can be employed in a number of chemical processes. Diisopropenylbenzene is normally synthesized by the dehydrogenation of diisopropylbenzene. Unfortunately in this dehydrogenation process a number of olefinic impurities are produced as by-products. This invention discloses a process for the separation of diisopropenylbenzene from these impurities and for recycling some of the impurities. In one embodiment of this invention this process comprises: (1) dehydrogenating diisopropylbenzene to form a dehydrogenation mixture containing diisopropenylbenzene and organic impurities, (2) continuously distilling said dehydrogenation mixture to separate said diisopropenylbenzene from said organic impurities, (3) fully hydrogenating said organic impurities to form a mixture of regenerated diisopropylbenzene and saturated organic impurities, and (4) fractionally distilling said mixture of regenerated diisopropylbenzene and saturated organic impurities under conditions sufficient to separate said regenerated diisopropylbenzene from said saturated organic impurities. The regenerated diisopropylbenzene can then be recycled for dehydrogenation with fresh diisopropylbenzene in the first step of the above described process.

REFERENCES:
patent: 2402740 (1946-06-01), Doumani et al.
patent: 2443217 (1948-06-01), Amos et al.
patent: 3100807 (1963-08-01), Hatfield et al.
patent: 3631213 (1971-12-01), Brewer
patent: 3652699 (1972-03-01), Soderquist et al.
patent: 4338476 (1982-07-01), Vickers et al.

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