Process for the reductive deposition of polyoxometallates

Chemistry: electrical and wave energy – Processes and products

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2041815, C25D 300, C25D 908, C25D 1302

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active

046345027

ABSTRACT:
A process for the reductive deposition of polyoxometallate complexes on supports. The process includes the steps of forming a solution of at least one polyoxometallate compound in a solvent, said compound having the formula A.sub.a (L.sub.l M.sub.m J.sub.z O.sub.y), adding a quantity of a support material having electronic conductivity to the solution, charging the solution containing the support material to an electrolytic cell in contact with the cathode thereof, the cell having a separate compartment for the anode, passing a current of from about 0.1 to about 500 mA/cm.sup.2 of electrode area through the cell whereby the support material receives a deposit of a polyoxometallate wherein the average oxidation state of the metals therein has been reduced to a valence greater than zero and, thereafter separating and recovering the support material carrying the reduced metallate complex.

REFERENCES:
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patent: 3703446 (1972-11-01), Haycock et al.
patent: 4092223 (1978-05-01), Kaufman
patent: 4222828 (1980-09-01), Zuurdeeg
patent: 4225322 (1978-09-01), Morcos
patent: 4272333 (1981-06-01), Scott et al.
patent: 4292144 (1981-09-01), Lepetit et al.
patent: 4411742 (1983-10-01), Donakowski et al.

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