Process for the production of...

Organic compounds -- part of the class 532-570 series – Organic compounds – Silicon containing

Reexamination Certificate

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Reexamination Certificate

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07348446

ABSTRACT:
A process for the production of trialkylsilyl (fluorosulfonyl)difluoroacetate by contacting (fluorosulfonyl)difluoroacetyl fluoride with siloxane. The amount of (fluorosulfonyl)difluoroacetic acid by-product in trialkylsilyl(fluorosulfonyl)difluoroacetate is reduced by contacting said mixture with trialkylsilyl halide.

REFERENCES:
patent: 5268511 (1993-12-01), Farnham
patent: WO 93/20085 (1993-10-01), None
William R. Dolbier Jr., et al. “Trimethylsilyl fluorosulfonyldifluoroacetate (TFDA): a new, highly efficient difluorocarbene reagent”, Journal of Fluorine Chemistry, 125 (2004) pp. 459-469.
Robin J. Terjeson et al., “Silver (Fluorosulfonyl)Difluoroacetate—A New Route to Fluorosulfonyl Esters”, Journal of Fluorine Chemistry, 42 (1989) pp. 187-200.
Feng Tian et al., “A Novel and Highly Efficient Synthesis of gem-Difluorocyclopropanes”, Organic Letters, vol. 2, No. 4, (2000) pp. 563-564.
W. R. Dolbier, Jr., et al., “Preparation and Use of a New Difluorocarbene Reagent, Trimethylsilyl 2-Fluorosulfonyl-2,2-Difluoroacetate: n-Butyl 2,2-Difluorocyclopropanecarboxylate”, Organic Syntheses, p. 172, vol. 80, (2003).
J. D. Citron, “Reactions of Group IVB Compounds with Acyl Fluorides”, Journal of Organometallic Chemistry, pp. 21-26, vol. 30, (1971).

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