Process for the preparation of α-chloroketones from...

Organic compounds -- part of the class 532-570 series – Organic compounds – Oxygen containing

Reexamination Certificate

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C568S316000, C568S346000, C568S348000, C568S397000, C568S020000, C564S123000, C564S161000, C564S209000

Reexamination Certificate

active

06924397

ABSTRACT:
The present invention relates to a process for the preparation of α-chloroketones from readily available alkyl esters by the reaction of a sulfoxonium ylide on said alkyl esters to generate a keto sulfoxonium ylide that is in turn treated with anhydrous HCl.

REFERENCES:
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patent: 6399793 (2002-06-01), Kronenthal et al.
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Carey, F.A. et al., Advanced Organic Chemistry, Fourth Edition, Part A: Structure and Mechanisms, Kluwer Academic/Plenum Publishers, publ., p. 473 (2000).
Chen, P. et al., “A Practical Method for the Preparation of α′-Chloroketones of N-Carbamate Protected-α-Aminoacids”, Tetrahedron Letters, vol. 38, No. 18, pp. 3175-3178 (1997).
Corey, E.J. et al., “A New Synthetic Approach to Medium-Sized Carbocyclic Systems”, J. Am. Chem. Soc., vol. 86, pp. 1641-1642 (1964).
DeGraw, J.I. et al., “α-Acetoxy and α-Halomethylketones from Acyloxosulfonium Ylides”, Tetrahedron Letters, No. 20, pp. 2501-2502 (1968).
Greene, T.W. et al., Protective Groups in Organic Synthesis, Third Edition, John Wiley & Sons, Inc., publ. (1999) (table of contents).
König, H. et al., “Über neue, stabile Schwefel-Ylide”, Chem. Ber., vol. 98, pp. 3733-3747 (1965).
Kowalski, C.J. et al., “Bromomethyl Ketones and Enolates: Alternative Products From Ester Homologation Reactions”, J. Org. Chem., vol. 50, pp. 5140-5142 (1985).
Kowalski, C.J. et al., “Ester Homologation Revisited: A Reliable, Higher Yielding and Better Understood Procedure”, J. Org. Chem., vol. 57, pp. 7194-7208 (1992).
Nagao, Y. et al., “A New Design for Chiral Induction: A Highly Regioselective Differentiation between Two Identical Groups in an Acyclic Compound Having a Prochiral Center”, J. Am. Chem. Soc., vol. 104, pp. 2079-2081 (1982).
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