Process for the preparation of metallosilicates of tetravalent l

Chemistry of inorganic compounds – Boron or compound thereof – Oxygen containing

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423326, 423328, 423329, 423330, 423331, 423332, 502 60, 502 62, 502 65, 502 71, 502 73, 502 77, 502202, C01B 3510

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active

046817476

ABSTRACT:
A molecular sieving metallosilicate is disclosed which comprises a complex represented in terms of mole ratios of oxides by the formula: ##STR1## wherein A is an ammonium, alkyl ammonium, alkyl phosphonium or alkyl arsonium ion; D is an alkali or alkaline earth metal ion or a mixture of two or more thereof; E is selected from the group consisting of Al, B, Mo, W, Fe, or a mixture of two or more thereof; M is a tetravalent metal selected from the Lanthanide or Actinide series; a is a number ranging from zero to about 25; b is a number ranging from zero to about 1.5; c is a number ranging from zero to about 0.3; d is a number ranging from about 20 to about 500; e is a number ranging from zero to about 200. The X-ray diffraction pattern for these metallosilicates indicates a ZSM-5 like crystalline structure. A method for making these metallosilicates, and a method for dehydrating and reforming methanol using these metallosilicates are disclosed.

REFERENCES:
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patent: 4163028 (1979-07-01), Tabak et al.
patent: 4188282 (1980-02-01), Tabak et al.
patent: 4564511 (1986-01-01), Desmond et al.
patent: 4576805 (1986-03-01), Chang et al.
patent: 4594146 (1986-06-01), Chester et al.

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