Process for the dehydrogenation of dehydrogenatable hydrocarbons

Chemistry of hydrocarbon compounds – Aromatic compound synthesis – Having alkenyl moiety – e.g. – styrene – etc.

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585906, C07C 402

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active

047177810

ABSTRACT:
Unsaturated hydrocarbons may be prepared by subjecting a dehydrogenatable hydrocarbon to dehydrogenation in the presence of a dehydrogenation catalyst. The effluent stream from this step, comprising unconverted hydrocarbons, dehydrogenated hydrocarbons, hydrogen and steam, may then be passed to a selective oxidation step in which the hydrogen is selectively oxidized in the presence of an oxygen-containing gas to the substantial exclusion of the oxidation of the hydrocarbons. The oxidation catalyst which is employed will comprise a Group VIII noble metal, a Group IVA metal and a Group IA or IIA metal composited on a metal oxide support. The metal oxide support such as alumina will possess a particular configuration having one or more open channels such as a tubular or cartwheel particle having an outside to inside diameter ratio of the channels ranging from 1.1 to 8 and having a ratio of shape surface to catalyst volume greater than [4D+2L] in which D is the largest representative diameter of the particle and L is the length of the particle.

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