Process for the continuous production of functionalized polymers

Synthetic resins or natural rubbers -- part of the class 520 ser – Synthetic resins – Treating polymer containing material or treating a solid...

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528392, 528483, 528487, 528495, 528497, 528499, 5253317, 5253333, 5253337, 5253338, 5253339, 525383, C08F 800, C08F 600, C08G 6700, C08J 300, C07C 6700

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060374454

ABSTRACT:
A continuous process for functionalizing polymers is disclosed, wherein (A) a liquid comprising the polymer and a gas comprising a functionalizing agent are continuously introduced into a dispersing zone operated in laminar flow with high intensity mixing of the liquid and the gas under functionalization conditions, wherein the mixing is conducted for a period of the dispersing zone residence time at a shear rate effective to form a stable gas-liquid dispersion in which the gas is substantially dissolved or dispersed in the liquid for functionalization, and wherein the shear rate is less than about 5 s.sup.-1 for no more than about 30% of the residence time; (B) the gas-liquid dispersion is continuously passed to a blending zone operated in laminar flow with low intensity mixing under functionalization conditions, wherein the mixing is conducted at a shear rate effective to further dissolve the gas into the liquid for further functionalization; and (C) continuously recovering functionalized polymer. The process can be used to carbonylate unsaturated polymers, and is particularly useful in reacting unsaturated polymers with carbon monoxide in the presence of a catalyst and a co-reactant selected from water, H.sub.2 S, alcohols, and thiols to produce functionalized polymer containing carboxylic (thio)acid or carboxylic (thio)ester functional groups.

REFERENCES:
patent: 2831877 (1958-04-01), Koch
patent: 5409672 (1995-04-01), Cetinkaya
patent: 5629434 (1997-05-01), Cusumano et al.
patent: 5650536 (1997-07-01), Dankworth et al.
Meyer, Chris F., "Laminar Flow Static Mixing-Design and Scaleup Criteria", 1991 AlChE Annual Meeting, Los Angeles, Nov. 17-22, 1991: Session 119, Industrial Mixing and Scaleup.
Streiff, F.A. et al., "Don't Overlook Static-Mixer Reactors", Chemical Engineering, Jun. 1994, pp. 76-82.
H. Bahraman, "Koch Reactions", Chapter 5, New Syntheses with Carbon Monoxide, edited by J.Falbe, Springer-Verlag, New York, 1980.
Fleischli, Markus et al., Neue Erkenntnisse zum Mischen und Dispergieren von Flussigkeiten it grossen Viskositatsunterschieden in statischen Mischern, Chem.-Ing.-Tech., 62 (1990), No. 8, pp650,653 and 654.

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