Process for selectively acylating immunomycin

Chemistry: molecular biology and microbiology – Micro-organism – tissue cell culture or enzyme using process... – Preparing heterocyclic carbon compound having only o – n – s,...

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435118, 435136, 435198, C12P 1718, C12P 1716, C12P 740, C12N 920

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active

052100308

ABSTRACT:
Described is a new process for selectively acylating FK-506 type immunosuppressant macrolides, including immunomycin (FK-520), in the C-32 position, under novel conditions utilizing an immobilized lipase enzyme, an acyl donor, and a dry, non hydroxylic organic solvent. The enzyme is absorbed onto a solid support and the enzyme/support catalyzes the C-32 acylation. The enzyme/support complex can then be filtered from the reaction mixture and, recycled for use.

REFERENCES:
patent: 3244592 (1966-05-01), Arai
patent: 4894366 (1990-01-01), Okuhara et al.
Bianchi et al., J. Org. Chem., vol. 53, pp. 5531-5534, 1988.
J. Antibiotics, A15, pp. 231-232, by Arai, et al.

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