Process for realuminating zeolites

Chemistry of inorganic compounds – Silicon or compound thereof – Oxygen containing

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423329, 502 63, 502 85, 502 86, C01B 3334

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active

051184826

ABSTRACT:
The instant invention comprises a process for increasing the framework aluminum content of a framework aluminum deficient zeolite containing non-framework aluminum by contacting said zeolite with an aqueous basic solution at a temperature greater than about 25.degree. C. Preferably the aqueous solution comprises ammonium and/or alkali metal hydroxides dissolved in water and the contact temperature ranges between about 60.degree. C. and about 90.degree. C. The instant invention also relates to the zeolites thus prepared by the instant process.

REFERENCES:
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patent: 4468475 (1984-08-01), Kuehl
patent: 4477582 (1984-10-01), Miale
patent: 4478950 (1984-10-01), Chu
patent: 4513091 (1985-04-01), Chang
patent: 4550092 (1985-10-01), Chang et al.
patent: 4563435 (1986-01-01), Chu et al.
patent: 4594333 (1986-06-01), Chang et al.
patent: 4837398 (1989-06-01), Chang et al.
patent: 4871702 (1989-10-01), Chang et al.
patent: 4943545 (1990-07-01), Chang et al.
Liu et al., "Hydrothermal Isomorphous Insertion of Aluminium into the Framework of Zeolite Y: A Convenient Method of Modifying the Siting of Al and Si in Faujastic Catalyst," J. Chem. Soc. Commun., pp. 582-584, 1986.
Bexman, "On the Efficiency of Insertion of Aluminium into the Framework of Y-type Zeolite by the Hydrothermal Process of Liu, Klinowski, and Thomas," J. Chem. Soc., Chem. Commun., p. 1562, 1987.
Sulikowski, "Structural and Catalytic Consequences of Isomorphous Substitution of Silicon by Aluminium and vice versa in the Framework of Pentasil Zeolites," J. Chem. Soc., Chem. Commun., p. 1521, 1987.
Breek et al, "Zeolite Chemistry IV--Evidence for the Elimination and Subsequent Reinsertion of Framework Aluminum During the Stabilization of NH.sub.4 +-Exchanged Zeolite X," Proceedings of the Fifth International Conference on Zeolites, pp. 335-343, 1980.
Engelhardt et al., "A Reexamination of the Hypothesis of Breck and Skeels Concerning the Reinsertion of Aluminum in the Framework of Dealuminated Y Zeolites," J. of Catalysis 88, pp. 513-515, 1984.
Chang et al., "Insertion of Aluminium into High-silica-content Zeolite Framework," J. Chem. Soc., Faraday Trans. I, 81, pp. 2215-2224, 1985.
Anderson, et al., "Alumination of Highly Siliceous Zeolites," J. Chem. Soc., Chem. Commun., pp. 1596-1597, 1984.

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