Process for producing ultra-pure plutonium-238

Specialized metallurgical processes – compositions for use therei – Processes – Producing or treating free metal

Reexamination Certificate

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C376S170000, C376S182000

Reexamination Certificate

active

06896716

ABSTRACT:
A method for producing ultra-pure Pu-238 is provided. The method comprises the steps of short-term irradiating Am-241 targets with a high, thermal neutron flux greater than 6.5×1014neutrons cm−2s−1and more preferably greater than 1×1015neutrons cm−2s−1for a predetermined period of time preferably from 20 days to 30 days and more preferably approximately 25 days to convert a substantial fraction of the Am-241 to Cm-242, e.g., approximately 0.555 g of Cm-242 per g of Am-241 charged, thereafter promptly chemically separating the produced Cm-242, preferably within 10 days to 20 days of the irradiation cycle of the Am-241 targets and more preferably within about 15 days of the irradiation cycle of the Am-241 targets, and recovering the ultra-pure Pu-238 decay product of the separated Cm-242.

REFERENCES:
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patent: 2975113 (1961-03-01), Maret
patent: 3147109 (1964-09-01), Knighton et al.
patent: 3161462 (1964-12-01), Seaborg
patent: 3360477 (1967-12-01), Acree et al.
Ihle, H. et al; Isotopic Composition of Plutonium-238 from Americium-241 and Reactor Cross-Sections of Actinide Nuclides. 1972. J. Inorg. Nucl. Chem. 1972, vol. 34, pp. 2427-2437.*
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D. C. Stewart, et al., Data Relating to the Production of Transcurium Elements in High Neutron Fluxes, ANL 6932, Sep. 1, 1964 pp 5-9.
Carolyn A. Mangeng, et al., Beneficial Uses of 241 Am, LA-10075-MS, May, 1984, pp 1-8.
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W.E. Bickford, Savannah River Site—Personal Communication.

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