Process for producing silicon carbide ceramic micro tube...

Chemistry of inorganic compounds – Silicon or compound thereof – Binary compound

Reexamination Certificate

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Reexamination Certificate

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07964171

ABSTRACT:
An improved process for producing a silicon carbide ceramic micro tubes (SiC micro tube) from a silicon-based polymer fiber by applying an ionizing radiation such that the surface part of the fiber selectively undergoes oxidative crosslinking, extracting the uncrosslinked core part of the fiber with an organic solvent to form a hollow fiber, and firing it in an inert gas is characterized by using a polymer blend of polycarbosilane and polyvinylsilane as the silicon polymer or applying the ionizing radiation to the silicon-based polymer fiber as it is cooled. The two methods may be performed either individually or in combination to produce tubes with their wall thickness controlled at a desired value in the range of 2-10 μm although this has been impossible to achieve in the prior art.

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Idesaki et al, Application of electron beam curing for silicon carbide fiber syntheisi from blend polymer of polycarbosilane and polyvinylsilane, 2001, Radiation Physics and Chemistry, 60, pp. 483-487.
Idesaki, et al. “Fine silicon carbide fibers synthesized from polycarbosilane-polyvinylsilane polymer blend using electron beam curing”, Journal of Materials Science 36(2001), pp. 357-362.
Idesaki, et al. “Application of electron beam curing for silicon carbide fiber synthesis from blend polymer of polycarbosilane and polyvinylsilane”, Radiation Physics and Chemistry 60(2001), pp. 483-487.
Idesaki, et al. “Fine SiC fiber synthesized from organosilicon polymers: relationship between spinning temperature and melt viscosity of precursor polymers”, Journal of Materials Science 36(2001), pp. 5565-5569.
Narisawa, et al. “Thermal oxidation crosslinking in the blended precursors of organosilicon polymers containing polyvinylsilane with polycarbosilane”, Journal of Materials Science 33(1998), pp. 2663-2666.
Narisawa et al. “Use of Blended Precursors of Poly(vinylsilane) in Polycarbosilane for Silicon Carbide Fiber Synthesis with Radiation Curing”, J. Am. Ceram. Soc., 82 [4] (1999), pp. 1045-1051.
Japanese Office Action dated Nov. 12, 2009 issued in corresponding Japanese Patent Application 2004-331648.

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