Process for preparing trioxepane composition and use thereof...

Catalyst – solid sorbent – or support therefor: product or process – Catalyst or precursor therefor – Organic compound containing

Reexamination Certificate

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C525S050000, C525S256000, C525S387000, C549S266000

Reexamination Certificate

active

07825059

ABSTRACT:
Process to prepare a trioxepane compound of the following formula (I) comprising less than 3.5 wt % of dialkyl peroxide based on the total amount of peroxides, said process comprising the steps of reacting a glycol compound of the formula R3CHOH—CH2—C(CH3)2OH with hydrogen peroxide in the presence of an acid to form a glycol hydroperoxide, purifying the glycol hydroperoxide, reacting the purified glycol hydroperoxide with a ketone or aldehyde of the formula R1R2CO in the presence of an acid to form the trioxepane compound, and purifying the trioxepane compound, wherein R1, R2, and R3are independently selected from hydrogen and a substituted or unsubstituted hydrocarbyl group, with the proviso that if R1and R2are both methyl groups, R3is not hydrogen. Initiator compositions comprising the so-prepared trioxepane compound are characterized by a high safe processing temperature in combination with a good crosslink efficiency.

REFERENCES:
patent: WO 98/50354 (1998-11-01), None
patent: WO 9850354 (1998-11-01), None
Adam et al. [“1,2,4-Trioxepanes: Synthesis and Mass Spectral Behaviour,'” Journal of the Chemical Society, Chemical Communications, (13), 798-9, (1972)].
Kirk-Othmer [The Encyclopedia of Chemical Technology, 3rd Edition, vol. 17, p. 57, (1982)].
Waldemar, Adam, et al., “1,2,4-Trioxepanes: Synthesis and Mass Spectral Behaviour,”Journal of the Chemical Society, Chemical Communications, (13), 798-9, (1972).
Kirk-Othmer, The Encyclopedia of Chemical Technology, 3rdEdition, vol. 17, p. 57, (1982).

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