Process for preparing certain 1-lower alkanoyl or benzoyl-4-(low

Organic compounds -- part of the class 532-570 series – Organic compounds – Heterocyclic carbon compounds containing a hetero ring...

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546314, C07D21182

Patent

active

046819444

ABSTRACT:
There is described a novel process for preparing 4-pyridinylmethyl ketones of formula (I) ##STR1## wherein R is alkyl, aryl or aralkyl. The process involves hydrolysis of a compound ##STR2## generated by reaction of an acylating agent with 4-methylpyridine. The acylating agent may be selected from compounds of formula R-CO-X and R-CO-O-CO-R where R is as defined above and X represents halogen. Compounds of formula I have utility in the preparation of a variety of products, including pharmaceutically active 1,2-dihydro-6-R-2-oxo-5 pyridinyl compounds.

REFERENCES:
patent: 4347363 (1982-08-01), Singh
patent: 4413127 (1983-11-01), Singh
patent: 4417054 (1983-11-01), Gelotte
patent: 4469871 (1984-09-01), Gelotte
Anders et al., Chemische Berichte, vol. 116(9), pp. 3192-3201, Sep. 1983.
March, Advanced Organic Chemistry, Reactions, Mechanisms and Structure, Second Edition, p. 441, McGraw-Hill Pub. QD 251 M2 1977 C.5.
Gutsche and Voges, "Acylation and Other Reactions of 2- and 4-Pyridinylacetonitriles", Sep. 1967, pp. 2685-2689.

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