Process for preparing 2-fluoro-3-oxoalkylcarboxylic acid ester

Organic compounds -- part of the class 532-570 series – Organic compounds – Carboxylic acid esters

Reexamination Certificate

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Reexamination Certificate

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07019162

ABSTRACT:
A process for producing a 2-fluoro-3-oxoalkylcarboxylic acid ester by fluorinating 3-oxoalkylcarboxylic acid ester with a fluorine gas is provided. The process is characterized in that the concentration of 3-oxoalkylcarboxylic acid ester in the reaction mixture for fluorination is maintained at 3 wt % or higher. Also provided is a process for purifying 2-fluoro-3-oxoalkylcarboxylic acid ester characterized in that 2-fluoro-3-oxoalkylcarboxylic acid ester is produced at high yield and with less impurities by washing fluorinated 3-oxoalkylcarboxylic acid ester with 3 or more times as much water as the amount of reaction mixture. According to the processes of the present invention, not only is the generation of unwanted by-products minimized, but fluorinated 3-oxoalkylcarboxylic acid ester can be purified in an efficient manner. Thus, the present invention permits efficient production of considerably pure 2-fluoro-3-oxoalkylcarboxylic acid ester, a useful intermediate material in the production of various medical and agricultural agents.

REFERENCES:
patent: 0 891 962 (1999-01-01), None
patent: 9-255611 (1997-09-01), None
patent: 2001-354622 (2001-12-01), None
patent: 97/35824 (1997-10-01), None
patent: 01/30740 (2001-05-01), None
Chambers et al, Tetrahedron, Direct Fluorination of 1,3-Dicarbonyl Compounds, 1995, 52(1), pp. 1-8.

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