Polymethylaluminoxane preparation, method of producing the...

Organic compounds -- part of the class 532-570 series – Organic compounds – Aluminum containing

Reexamination Certificate

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C556S182000, C502S103000, C502S152000, C526S160000, C526S165000

Reexamination Certificate

active

07910764

ABSTRACT:
A polymethylaluminoxane preparation exhibiting excellent storage stability with a high yield is provided. A polymethylaluminoxane preparation is formed by thermal decomposition of an alkylaluminum compound having an aluminum-oxygen-carbon bond, the alkylaluminum compound being formed by a reaction between trimethylaluminum and an oxygen-containing organic compound. In this preparation,(i) the oxygen-containing organic compound reacting with trimethylaluminum is an aliphatic or aromatic carboxylic acid represented by the general formula (I),in-line-formulae description="In-line Formulae" end="lead"?R1—(COOH)n  (I),in-line-formulae description="In-line Formulae" end="tail"?wherein R1represents a hydrocarbon group of C1-C20 straight or branched alkyl groups, alkenyl groups or aryl groups, and n represents an integer of 1 to 5;(ii) a mole fraction of methyl groups originating from trimethylaluminum, relative to the total moles of methyl groups existing in the generated polymethylaluminoxane preparation is not more than 26 mol %; and(iii) the generated polymethylaluminoxane preparation has a viscosity of not more than 2.1×10−3Pa·sec at 40° C.

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Supplementary European Search Report issued Sep. 22, 2009, in corresponding European Application No. 05 72 1138.
Henri Cramail et al., “New synthetic route to methylaluminoxane for ethylene polymerization in the presence of zirconocene”, XP-002545405, C.R. Chimie, May 2002, pp. 49-52.

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