Photoelectrochemical cells

Chemistry: electrical current producing apparatus – product – and – Deferred action type – Responsive to light

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204 56R, H01M 636

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active

043883826

ABSTRACT:
Photovoltaic devices are fabricated by forming a thin passivating layer, for example, an oxide layer on a semiconductor material. The passivating layer on the semiconductor material is then contacted with an electrolyte such as an electrolyte containing vanadium ions. The resulting electrolyte/passivating layer/semiconductor (EPLS) structure exhibits excellent solar conversion efficiencies and good stability.

REFERENCES:
patent: 4343870 (1982-08-01), Heller et al.
A. Heller, et al., "11.5% Solar Conversion Efficiency in the Photocathodically Protected p-InP/V.sup.3+ -V.sup.2+ -HCl/C Semiconductor Liquid Junction Cell", Appl. Phys. Lett., vol. 38, pp. 282-284 (1981).
M. J. Madou et al., "Photochemical Corrosion of Semiconductors for Solar Cells," SPIE, vol. 248, Role of Electro-Optics In Photovoltaic Energy Conversion, (1980), pp. 88-95.
D. S. Ginley, et al., "Interfacial Chemistry at p-GaP Photoelectrodes," J. Electrochem. Soc., vol. 129, pp. 2141-2145 (1982).
S. Gourgaud et al., "Semiconductor/Electrolyte Photoelectric Energy Conversion: The Use of a Molybdenum Oxide Coating to Avoid Corrosion," J. Electrochem. Soc., vol. 124, pp. 102-107 (1977).
H. Morisaki et al., "Iron-Oxide Coated n-Si as a Heterostructure Photoanode for the Photoelectrolysis of Water," Japan. J. Appl. Phys., vol. 19, pp. L148-L150 (1980).
Y. Nakato, et al., "Photo-Electrochemical Behaviors of Semiconductor Electrodes Coated with Thin Metal Films", Chem. Lett. pp. 883-886 (1975).
A. Heller et al., "An Efficient Photocathode for Semiconductor Liquid Junction Cells: 9.4% Solar Conversion Efficiency With p-InP/VCl.sub.3 -VCl.sub.2 -HCl/C", J. Am. Chem. Soc., vol. 102, pp. 6535-6556 (1980).
A. M. Van Wezema et al., "Study of the Schottky Barrier at the n- And p-Type InP Electrode/Electrolyte Interface," J. Electroanal. Chem., vol. 87, pp. 105-109 (1978).
A. A. K. Vervaet et al., "Some Electrochemical Processes at the n- And P-InP Electrodes", J. Electroanal. Chem., vol. 91, pp. 133-136 (1978).

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