Pharmaceutical composition of F(ab1)2 antibody fragments and...

Drug – bio-affecting and body treating compositions – Immunoglobulin – antiserum – antibody – or antibody fragment,... – Binds hormone or other secreted growth regulatory factor,...

Reexamination Certificate

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C424S177100, C424S809000, C435S068100, C435S269000, C436S547000, C530S389100, C530S389200, C530S390500, C530S421000

Reexamination Certificate

active

06709655

ABSTRACT:

FIELD OF INVENTION
The present invention is directed to a pharmaceutical composition comprising F(ab′)
2
antibody fragments that are preferably free from albumin and of whole antibodies and also substantially free of pyrogens, and an effective amount of a pharmaceutically acceptable carrier. It is also directed to a method for the preparation of a pharmaceutical composition comprising F(ab′)
2
antibody fragments using serum or blood plasma of a mammal that has been previously immunized as a source of antibodies. The serum or blood plasma is digested with an enzyme, pepsin, followed by separation and purification until the pharmaceutical composition of F(ab′)
2
fragments are free of albumin and complete antibodies, and substantially free of pyrogens.
BACKGROUND
Antibodies are proteins of a globulin type known as immunoglobulins that are present in blood serum as a response of the immune system to the invasion of some foreign substance or organism, and are characterized for specifically combining with those substances that are foreign to the organism, neutralizing them and precipitating them so that they are removed from the circulation. Various industrial applications have been developed with them for the diagnosis, monitoring, prevention and treatment of different ailments.
In regions where, due to climatic conditions, venomous animals abound, antibodies have been given a special use to combat the venom and a large number of doses are applied when treating patients with scorpion, spider and snake stings or bites, principally. At present, a use that is gaining in importance is as a treatment for auto-immune diseases like rheumatoid arthritis, immune-dependent diabetes mellitus, AIDS, hemophilic anaemias, rheumatic fever, multiple sclerosis, thyroiditis and psoriasis, among others. In these cases, anti-cytokine antibodies are applied either directly to the patient or by treating blood that has been taken from and is subsequently re-fed to the patient, with the purpose of removing the cytokines generated by the organism itself in response to the ailment which, if they are not removed, would finally cause extremely troublesome symptoms (see U.S. Pat. No. 5,888,511 and 4,940,670).
There are several kinds of immunoglobins, known as IgG, IgN, IgD, IgA and IgE, of which IgG are the most abundant in the blood circulation and correspond to a mature immune response and therefore include the vast majority of antibodies that are commercially produced. All the IgG have the same general structure (which can be seen in
FIG. 1
) they are composed of four polypeptide chains, two that are heavy (H) and two light (L) which are joined together by disulfide bridges. The two heavy chains, in turn, are joined together by two other disulfide bridges known as the hinge region, approximately half way along the chains. A little closer to the amino terminal region, each heavy chain is joined by a disulfide bridge with a light chain. Each heavy chain has three constant regions, C
H
1, C
H
2, and C
H
3, the last two in the carboxy terminal region (before the hinge) and the first in the amino terminal region (immediately after the hinge) and a Variable region (VH) in the amino terminal end, while each light chain has only one constant region, CL, in the carboxy terminal end and one variable region, VL, in the amino terminal end.
When the IgG is digested enzymatically, different fragments are obtained depending on the enzyme used, that is, if papain is used, three fragments are obtained, the crystallizing fragment (Fc) and two antigen-binding fragments (Fab) and, if pepsin is used, one F(ab′)
2
fragment is obtained, while the crystallizing fragment is digested. The foregoing is due to the fact that papain cuts the heavy chains immediately after the hinge (towards the amino terminal region), while pepsin cuts them before the hinge (towards the carboxy terminal region). Fab and F(ab′)
2
are the fragments that conserve their capacity to specifically bind to the antigen that gave rise to them and F(ab′)
2
also precipitates them, while the Fc antibody fraction normally acts as a marker signal for macrophages and the activation of lymphocytes for the recognition and phagocytosis of the antigen-antibody complex.
The Fc fragment comprises the antigenic determinants of the antibody in such a way that, when a patient is administered whole antibodies generated in some animal of another species, the patient generates an immune response against these antigenic determinants giving rise to varied adverse secondary responses that can even include anaphylactic shock.
These problems are significantly reduced when the antibodies are previously digested with papain or pepsin and only the resulting purified Fab or F(ab′)
2
fragments are administered.
The use of Fab or F(ab′)
2
fragments has another advantage that is known as the concept of distribution volume, which is simply the volume of the body in which a determined drug is dissolved. This volume can refer to the circulating blood alone, as is the case of IgG, or can include a larger part of body water in the case of the fragments. For this reason, as Fab and F(ab′)
2
have a greater corporal volume they can neutralize toxins lodged in various tissues, not only in the blood, they can even cross the blood/brain barrier in both direct ions and be used to neutralize or eliminate neurotoxins.
The use of F(ab′)
2
has a particular advantage over Fab in that they are retained far longer in the organism because they have double the molecular weight and, moreover, they conserve their capacity to precipitate the antigen in physiological conditions as well as maintaining a size that allows them access to a distribution volume that is sufficient for treatment purposes.
As the F(ab′)
2
fragments conserve the main characteristics of the antibodies, the applications of the antibodies extend to F(ab′)
2
fragments, with the additional advantage that because they lack, the Fc fragment, recognition as foreign by the organism of the patient they are being administered to is less, thus providing greater tolerance to application and reducing the possibility of secondary reactions, which is particularly useful for prolonged treatments such as those applied in autoimmune diseases.
It has been known for many years that soluble proteins (particularly serous proteins) lose solubility as the concentration of neutral salts (such as ammonium and sodium sulfates) in the solution increases. In this way, for example, euglobulin precipitates with 13.5% sodium sulfate, pseudoglobulin with 17.4% and pseudoglobulin 2 with 21.3%. This fact has been used to partially purify antibodies from serum or plasma.
Several approaches in the production of antibodies and their fragments have been reported in the literature. For example, in U.S. Pat. No. 4,849,352, Sullivan et al. claims the production of both Fab fragments through the digestion of antibodies with papain immobilized in polyacrylamide and F(ab′)
2
fragments through the digestion of antibodies with immobilized pepsin, obtaining Fab and Fc or F(ab′)
2
fragments and subsequently purifying the fragments through immunoaffinity, passing them through a polyacrylamide sieve containing the specific antigen of the antibodies in question and later recovering the Fab or F(ab′)
2
fragments that have specifically bound to the molecules in the sieve, with some strongly ionic solution. In spite of the purity of the fragments in question that are obtained, in the large scale commercial production of preparations of antibody fragments, both the use of immobilized enzymes for digestion and immobilized antigens for purification could prove to be extremely expensive.
Furthermore, in spite of the their use in producing antibody fragments generated against pure substances, when it is a question of antibodies generated against venoms, that are mixtures of a large amount of toxins, many of which have a biological effect, it is not economically feasible to obtain the antigenic siev

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