Drug – bio-affecting and body treating compositions – Designated organic active ingredient containing – Acyclic nitrogen double bonded to acyclic nitrogen – acyclic...
Reexamination Certificate
2000-11-27
2003-02-04
Pryor, Alton (Department: 1616)
Drug, bio-affecting and body treating compositions
Designated organic active ingredient containing
Acyclic nitrogen double bonded to acyclic nitrogen, acyclic...
Reexamination Certificate
active
06514954
ABSTRACT:
The present invention relates to a composition which comprises a pesticidal active compound combination, a method of controlling pests with this composition, a process for the preparation of the composition, its use and plant propagation material treated with it, and the use of a compound of the following formula (A) for the preparation of the composition.
Certain mixtures of active compounds are proposed for pest control in the literature. However, the biological properties of these mixtures of known compounds are not completely satisfactory in the field of pest control, and for this reason there is a need to provide further mixtures having synergistic pest control properties, in particular for controling of insects and representatives of the order Acarina. This object is achieved according to the invention by providing the present composition.
The invention accordingly relates to a composition for controlling insects or representatives of the order Acarina, which comprises a combination of variable amounts of one or more compounds of the formula
in which
A is an unsubstituted or, depending on the possibility of substitution on the ring system, mono- to tetrasubstituted, aromatic or non-aromatic monocyclic or bicyclic heterocyclic radical, in which the substituents of A are chosen from the group consisting of C
1
-C
3
alkyl, C
1
-C
3
alkoxy, halogen, halo-C
1
14
C
3
alkyl, cyclopropyl, halocyclopropyl, C
2
-C
3
alkenyl, C
2
-C
3
alkynyl, halo-C
2
-C
3
alkenyl, halo-C
2
-C
3
alkynyl, halo-C
1
-C
3
alkoxy, C
1
-C
3
-C
3
alkylthio, halo-C
1
-C
3
alkylthio, allyloxy, propargyloxy, allylthio, propargylthio, haloallyloxy, haloallylthio, cyano and nitro;
R is hydrogen, C
1
-C
6
alkyl, phenyl-C
1
-C
4
alkyl, C
3
-C
6
cycloalkyl, C
2
-C
6
alkenyl or C
2
-C
6
alkynyl; and
X is N—NO
2
or N—CN,
in the free form or in salt form, if appropriate tautomers, in the free form or salt form, and one or more of the compounds:
(I) azamethiphos;
(XII) furathiocarb;
(II) chlorfenvinphos;
(XIII) isazofos;
(III) cypermethrin, cypermethrin high-cis;
(XIV) jodfenphos;
(IV) cyromazin;
(XV) kinoprene;
(V) diafenthiuron;
(XVI) lufenuron;
(VI) diazinon;
(XVII) methacriphos;
(VII) dichlorvos;
(XVIII) methidathion;
(VIII) dicrotophos;
(XIX) monocrotophos;
(IX) dicyclanil;
(XX) phosphamidon;
(X) fenoxycarb;
(XXI) profenofos;
(XI) fluazuron;
(XXII) diofenolan;
(XXIII) a substance obtainable from the Bacillus thuringiensis strain GC91
or from NCTC11821;
(XXIV) pymetrozine;
(XXVIII) quinalphos;
(XXV) bromopropylate;
(XXIX) tau-fluvalinate;
(XXVI) methoprene;
(XXX) thiocyclam; or
(XXVII) disulfuton;
(XXXI) thiometon;
and at least one auxiliary.
The compounds of the formula (A) are described in EP-A-580553.
(I) S-6-chloro-2,3-dihydro-2-oxo-1,3-oxazolo[4,5-b]pyridin-3-ylmethyl O,O-dimethyl phosphorothioate (azamethiphos) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 44;
(II) 2-chloro-1-(2,4-dichlorophenyl)vinyl diethyl phosphate (chlorfenvinphos) is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 174;
(III) (RS)-&agr;-cyano-3-phenoxybenzyl (1RS)-cis-trans-3-(2,2-dichlorvinyl)-1,1-dimethylcyclo-propanecarboxylate (cypermethrin, cypermethrin high-cis) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 208;
(IV) N-cyclopropyl-1,3,5-triazine-2,4,6-triamine (cyromazin) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 217;
(V) 1-tert-butyl-3-(2,6-diisopropyl-4-phenoxyphenyl)thiourea (diafenthiuron) is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 294;
(VI) O,O-diethyl O-2-isopropyl-6-methylpyrimidin-4-yl-phosphorothioate (diazinon) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 243;
(VII) 2,2-dichlorovinyl dimethyl phosphate (dichlorvos), is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 259;
(VIII) (E)-2-dimethylcarbamoyl-1-methylvinyl dimethyl phosphate (dicrotophos) is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 322;
(IX) 5-cyano-2-cyclopropylamino-4,6-diaminopyrimidine (dicyclanil) is known from EP-A-244360;
(X) ethyl 2-(4-phenoxyphenoxy)ethylcarbamate (fenoxycarb) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 375;
(XI) 1-[4-chloro-3-(3-chloro-5-trifluoromethyl-2-pyridylox)phenyl]-3-(2,6-difluorobenzoyl)-urea (fluazuron) is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 475;
(XII) butyl 2,3-dihydro-2,2-dimethylbenzofuran-7-yl N,N′-dimethyl-N,N′-thiodicarbamate (furathiocarb) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 448;
(XIII) O-5-chloro-1-isopropyl-1H-1,2,4-triazol-3-yl O,O-diethyl phosphorothioate (isazofos) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 502;
(XIV) O-2,5-dichloro-4-iodophenyl O,O-dimethylphosphorothioate Godfenphos) is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 1102;
(XV) prop-2-ynyl (±) (E,E)-3,7,11-trimethyidodeca-2,4-dienoate (kinoprene) is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 1102;
(XVI) (R,S)-1-[2,5-dichloro-4-(1,1,2,3,3,3-hexafluoropropoxy)phenyl]-3-(2,6-difluorobenzoyl)-urea (lufenuron) is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 628;
(XVII) methyl (E)-3-(dimethoxyphosphinothioyloxy)-2-methylacrylate (methacriphos) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 562;
(XVIII) S-2,3-dihydro-5-methoxy-2-oxo-1,3,4-thiadiazol-3-ylmethyl O,O-dimethyl phosphorodithioate (methidathion) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 567;
(XIX) dimethyl (E)-1-methyl-2-(methylcarbamoyl)vinyl phosphate (monocrotophos) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 597;
(XX) b
2
-chloro-2-diethylcarbamoyl-1-methylvinyl dimethyl phosphate (phosphamidon) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 679;
(XXI) O-4-bromo-2-chlorophenyl O-ethyl S-propyl phosphorothioate (profenofos) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 705;
(XXII) a mixture of 50 to 80% of (2RS,4SR)-4-(2-ethyl-1,3-dioxolan-4-ylmethoxy)phenyl phenyl ether and 50 to 20% of (2RS,4RS)-4-(2-ethyl-1,3-dioxolan-4-ylmethoxy)phenyl phenyl ether (diofenolan) is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 363;
(XXIII) a substance obtainable from the
Bacillus thuringiensis
strain GC91 or a substance obtainable from the
Bacillus thuringiensis
strain NCTC11821 is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 62;
(XXIV) 2,3,4,5-tetrahydro-3-oxo-4-[(pyridin-3-yl)-methyleneamino]-6-methyl-1,2,4-triazine (pymetrozine) is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 868; and
(XXV) isopropyl 4,4′-dibromobenzilate (bromopropylate) is known from The Pesticide Manual, 9
th
Edition (1991), The British Crop Protection Council, London, page 99,
(XXVI) isopropyl (E,E)-(R,S)-11-methoxy-3,7,11-trimethyldodeca-2,4-dienoate (methoprene) is known from The Pesticide Manual, 10
th
Edition (1994), The British Crop Protection Council, London, page 680;
(XXVII) O,O-diethyl S-2-ethylthioethyl phosphorodithioate
Maienfisch Peter
Senn Robert
Wyss Peter
Allen Rose M.
Pryor Alton
Syngenta Crop Protection Inc.
Teoli, Jr. William A.
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