On-column derivatization in capillary electrophoresis

Chemistry: electrical and wave energy – Processes and products – Electrostatic field or electrical discharge

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204299R, G01N 2726, G01N 27447

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active

053186800

ABSTRACT:
An on-column derivatization scheme where a liquid or solid labeling reagent is provided in a capillary to react chemically with a sample in order to label the sample. Electrophoretic separation may be carried out immediately thereafter to simplify the derivatization, separation and detection process. By localizing the labeling process to a small area within the capillary, fast kinetics and high reaction yield are achieved.

REFERENCES:
patent: 5045172 (1991-09-01), Guzman
patent: 5110431 (1992-05-01), Moring
Stephen L. Pentoney, Jr. et al., "On-Line Connector for Microcolumns: Application to the On-Column o-Phthaldialdehyde Derivativation of Amino Acids Separated by Capillary Zone Electrophoresis", Analytical Chemistry, vol. 60, No. 23 (Dec. 1, 1988) 2625-2629.
Richard M. Caprioli et al., "Coupling Cappillary zone Electrophoresis and Continuous-Flow Fast Atom Bombardment Mass Spectrometry for the Analysis of Peptide Mixtures", Journal of Chromatography, 480 (1989).
U. R. Tjaden, N. J. Reinhoud, and J. Vander Greef, "On-Line Derivatization In High Performance Capillary Electrophoresis", poster presentation at The Thirteenth Symposium on Column Liquid Chromatography, Stockholm, Sweden, Jun. 25-30, 1989.
"A Polymeric Reagent for Derivatization of Weak Nucleophiles in HPLC-UV", by Bourque and Krull, Journal of Chromatographic Science, 29:489-496, Nov. 1991.
"The Use of a Concentration Step to Collect Urinary Components Separated by Capillary Electrophoresis . . . ", by Guzman et al., Journ. of Liq. Chromatography 14(5):997-1015, 1991.
"The Use of On-Line Sample Concentration to Increase the Sensitivity of Capillary Electrophoresis", presented by Merion, et al., Mass. HPCE'91.
"Solid-Phase Reagent Containing the 3,5-Dinitrophenyl Tag for the Improved Derivatization of Chiral and Achiral Amines, . . . ", by Bourque et al., Journal of Chromatography, 537:123-152, 1991.
"On-Line Connector for Microcolumns: Application to the On-Column o-Phthaldialdehyde Derivatization of . . . ", by Pentoney, Jr. et al., Anal. Chem., 60:2625-2629, 1988.
"Capillary Isoelectric Focusing of Proteins in Uncoated Fused-Silica Capillaries Using Polymeric . . . ", by Mazzeo et al., Anal. Chem., 63:2852-2857, 1991.
"On-Line Derivatization in High Performance Capillary Electrophoresis", by Tjaden, et al., The Netherlands.
Patent Application Ser. No. 07/235,953 filed Aug. 24, 1988.

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