Neutral protic-salt electrolytes and protic-salt imbibed...

Chemistry: electrical current producing apparatus – product – and – With pressure equalizing means for liquid immersion operation

Reexamination Certificate

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C429S314000, C429S317000, C521S027000

Reexamination Certificate

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07833643

ABSTRACT:
A neutral protic salt electrolyte and a protic-salt imbibed polymer electrolyte membrane exhibiting high ionic conductivity and thermal stability at temperatures greater than 100° C. without requiring additional humidification systems or hydrating water is disclosed. The protic salt is the neutral product of acids and bases for which the proton transfer energy lies in the range from 0.5 to 1.5 eV. A polymer electrolyte membrane having the general formula:wherein A is a repeating unit in the main chain, B is a crosslinker chain, C is an end group, YZ is a neutralized couple at chain end, IL is an ionic liquid, and NP is a nanoparticle which absorbs the protic liquid yielding membranes that combine high mechanical strength with high conductivity. The present polymer electrolyte membrane is useful in high temperature fuel cells for automotive, industrial, and mobile communication applications.

REFERENCES:
patent: 2007/0006774 (2007-01-01), Rogers et al.
patent: 2009/0133746 (2009-05-01), Jin et al.
Kerres, J.A., “Development of ionomer membranes for fuel cells,” J. Membrane Sciences, 185, 3-27 (2001).
Nolte, R., Ledjeff, K., Bauer, M., and Mulhaupt, R., “Partially sulfonated poly (axylene ether sulfone)- A versatile proton conducting membrane material for modern energy conversion technologies,” J. Membrane Sciences, 83,211-220 (1993).
Xu, W. and Angell, C.A., “Solvent-Free Electrolytes with Aqueous Solution- Like Conductivities,” Science, 302, 422-425 (2003).
Kerres, J.A., “Development of ionomer membranes for fuel cells,” J. Membrane Sciences, 185, 3 (2001).

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