Mutated D-aminotransferase and method for producing...

Chemistry: molecular biology and microbiology – Micro-organism – tissue cell culture or enzyme using process... – Preparing alpha or beta amino acid or substituted amino acid...

Reexamination Certificate

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C435S069100, C435S193000, C435S320100, C435S252300, C435S325000, C536S023200

Reexamination Certificate

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07402412

ABSTRACT:
A D-aminotransferase can be modified so as to efficiently produce (2R, 4R)-monatin having high sweetness intensity from 4-(indol-3-ylmethyl)-4-hydroxy-2-oxoglutaric acid by substituting an amino acid at least at one of positions (positions 100, 180 to 183, 243 and 244) involved in efficiently producing the (2R, 4R)-monatin in an amino acid sequence of a wild-type D-aminotransferase represented in SEQ ID NO:2.

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patent: 6337190 (2002-01-01), Hwang et al.
patent: 6635749 (2003-10-01), Frankel
patent: 0 736 604 (1996-10-01), None
patent: WO 03/056026 (2003-07-01), None
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C.W. Holzapfel, “The Synthesis of A Gamma-Keto-Alpha-Amino Acid, A Key Intermediate in the Synthesis of Montain, A New Natural Sweetener”, Synthetic Communications, vol. 23, No. 18, pp. 2511-2526, 1993.
Database UniProt [Online] “D-Alanine Aminotransferase (EC 2.6.1.21) (D-Aspartate Aminotransferase) (D-Amino Acid Aminotransferase) (D-Amino Acid Transaminase) (DAAT)”, XP-002383319, Database accession no. DAAA—BACSH, Oct. 1, 1996.
P.W. Van Ophem, et al., “Catalytic Ability and Stability of Two Recombinant Mutants of D-Amino Acid Transaminase Involved in Coenzyme Binding”, Protein Science, 4, 1995, pp. 2578-2586, XP-002383317.
I.G. Fotheringham, et al., “Characterization of the Genes Encoding D-Amino Acid Transaminase and Glutamate Racemase, Two D-Glutamate Biosynthetic Enzymes ofBacillus sphaericusATCC 10208”, Journal of Bacteriology, vol. 180, No. 16, pp. 4319-4323, Aug. 1998.
S. Sugio, et al., “Crystal Structure of a D-Amino Acid Aminotransferase: How the Protein Controls Stereoselectivity”, Biochemistry, vol. 34, No. 30, pp. 9661-9669, 1995.
H.-S. RO, et al., “Site-Directed Mutagenesis of the Amino Acid Residues in Beta-Strand III (VAL30-VAL36) of D-Amino Acid Aminotransferase OB Bacillus SP. YM-1”, FEBS Letters, vol. 398, No. 2-3, pp. 141-145, Dec. 2, 1996.
K. Kishimoto, et al., “Role of Leucine 201 of Themostable D-Amino Acid Aminotransferase from A Thermophile, Bacillus SP. YM-1”, J. Biochem., vol. 117, No. 4, pp. 691-696, Apr. 1995.

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