Multinuclear half metallocene catalyst and preparation of...

Synthetic resins or natural rubbers -- part of the class 520 ser – Synthetic resins – Polymers from only ethylenic monomers or processes of...

Reexamination Certificate

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C526S160000, C526S161000, C526S172000, C526S346000, C526S347000, C526S347100, C502S103000, C502S117000, C502S152000, C502S155000, C556S052000, C556S055000, C556S001000

Reexamination Certificate

active

06894129

ABSTRACT:
The present invention relates to a catalyst for preparing vinyl aromatic polymer and styrene polymerization using the same, and particularly to a transition metal half metallocene catalyst with a novel structure for preparing syndiotactic styrene polymer having high activity, superior stereoregularity, high melting point and various molecular weight distributions and a process for preparing styrene polymer using the same. The present invention provides a multinuclear half metallocene compound in which two or more of transition metals of groups 3 to 10 on periodic table are connected through bridge ligand simultaneously containing π-ligand cycloalkandienyl group and σ-ligand functional group and its preparation, and a process for preparing styrene polymer using the compound as a catalyst. Polymers with various molecular weight distributions as well as vinyl aromatic polymer having predominant syndiotactic structure can be prepared with high activity using the multinuclear half metallocene catalyst.

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Y. Kim, et al., “New half-sandwich metallocene catalyst for polyethylene and polystyrene”, Journal of Organometallic Chemistry 634, 2001, pp. 19-24.
Y. Tianger, et al., “Recent Advances in Synthesis of Novel Half-Sandwich Group 4 Metallocene Complexes”, Chemical Journal on Internet, retrieved on Aug. 29, 2002.
Y. Kim, et al., New Half-Metallocene Catalysts Generating Polyethylene with Bimodal Molecular Weight Distribution and Syndiotactic Polystyrene, Macromol Rapid Commun., 22, 2001, pp. 573-578.
International Search Report; PCT/KR02/01317; Oct., 9, 2002.

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