Modification of polymer surfaces as radioisotope carriers

Surgery – Radioactive substance applied to body for therapy

Reexamination Certificate

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C404S001000, C404S001000

Reexamination Certificate

active

09657701

ABSTRACT:
A radioactive source is made by forming a polymer layer substantially free of inorganic polymers on a substrate material, and exposing the polymer layer to a radioactive isotope. The source is useful for inhibition of restenosis in coronary arteries after balloon angioplasty or stent implantation. In particular, a radioactive source of32P,90Y, or144Ce is deposited on a poly(ethylene terephtalate) (PET) substrate. The polymer substrate was first coated with pH-sensitive hydrogel and then adsorbed various amount of phosphoric acid (PA) in aqueous solutions. The substrate was immersed in32P,90YCl3or144CeCl3solutions, and then32P,90Y or144Ce was deposited on the surface as32PPO4,90YPO4or144Ce PO4. Two different polyurethanes were used to encapsulate and seal the deposited isotopes on the surface to minimize the leakage of the isotope.

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