Mixed metal oxide catalysts for the production of...

Catalyst – solid sorbent – or support therefor: product or process – Catalyst or precursor therefor – Metal – metal oxide or metal hydroxide

Reexamination Certificate

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C502S240000, C502S255000, C502S263000, C502S305000, C502S313000, C502S314000, C502S315000, C502S316000, C502S321000, C502S322000, C502S349000, C502S350000, C502S415000, C502S439000

Reexamination Certificate

active

11079038

ABSTRACT:
A catalyst for production of unsaturated aldehydes, such as methacrolein, by gas phase catalytic oxidation of olefins, such as isobutylene, contains oxides of molybdenum, bismuth, iron, cesium and, optionally, other metals. The catalyst has a certain relative amount ratio of cesium to bismuth, a certain relative amount ratio of iron to bismuth and a certain relative amount ratio of bismuth, iron, cesium and certain other metals to molybdenum and, optionally, tungsten. For a catalyst of the formula:in-line-formulae description="In-line Formulae" end="lead"?Mo12BiaWbFecCodNieSbfCsgMghZniPjOxin-line-formulae description="In-line Formulae" end="tail"?wherein a is 0.1 to 1.5, b is 0 to 4, c is 0.2 to 5.0, d is 0 to 9, e is 0 to 9, f is 0 to 2.0, g is from 0.4 to 1.5, h is 0 to 1.5, i is 0 to 2.0, j is 0 to 0.5 and x is determined by the valences of the other components, c:g=3.3–5.0, c:a=2.0–6.0 and (3a+3c+2d+2e+g+2h+2i)/(2×12+2b)=0.95–1.10.

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