Method of preparing an acid additional salt of delta-aminolevuli

Organic compounds -- part of the class 532-570 series – Organic compounds – Carboxylic acids and salts thereof

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C07C22900

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052849732

ABSTRACT:
An acid addition salt of .delta.-aminolevulinic acid is prepared in such a way that tetrahydrofurfurylamine (VI) is reacted with phthalic anhydride under an anhydrous condition to introduce a phthal group which protects amino group of tetrahydrofurfurylamine to give N-tetrahydrofurfuryl phthalimide (III), carbon atoms of the first- and fourth-positions of thus obtained N-tetrahydrofurfurylphthalimide (III) are oxidized at 80.degree. C. using sodium periodate as a oxidizing agent and ruthenium chloride hydrate as a catalyst to yield 5-phthalimidolevulinic acid (II), then the protecting group of 5-phthalimidolevulinic acid (II) is deprotected using an acid to prepare an acid additional salt of .delta.-aminolevulinic acid. The acid additional salt of .delta.-aminolevulinic acid is readily converted by neutralization by an alkali to .delta.-aminolevulinic acid, which is very useful as a precursor of Vitamin B.sub.12, heme and chlorophyll.

REFERENCES:
patent: 3846490 (1974-11-01), Aronova
patent: 4325877 (1982-04-01), Metcalf et al.
Tetrahedron Letters, vol. 25, No. 28, pp. 2977-2980, 1984.
Journal of the Chemical Society, Chemical Communications, vol. 17, pp. 753-754, 1978.
Agric. Biol. Chem., 55(6), 1687-1688, 1991, pp. 1687-1688.
Chem. Abstr., 113:114,653x (1990).

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