Method of phase transition, method for producing lead niobate-ba

Compositions: ceramic – Ceramic compositions – Titanate – zirconate – stannate – niobate – or tantalate or...

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501134, 501135, 252 629, 252500, 252518, 252521, 423592, 423598, 423622, 423632, 264 65, 264 66, C04B 3546, C04B 3548, C04B 3549, H01B 100

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051927233

ABSTRACT:
A method for producing a lead niobate-based complex oxide with an elevated proportion of pervoskite phase and lead niobate-based complex oxide produced by such method enables manufacture of small actuator or capacitor with an elevated dielectric constant k. Treatment of a raw material represented by a general formula Pb(A.sub.1/3 Nb.sub.#)x(ZN.sub.1/3 Nb.sub.2/3) yO.sub.3 or Pb(Fe.sub.1/2 Nb.sub.1/2)x(Zn.sub.1/3 Nb.sub.2/3) yO.sub.3 (wherein A is Mg or Ni; x is an atomic ratio in a range of 0-1; and y is an atomic ratio in a range of 1-0, with a relation x+y=1) and containing pyrochlore phase, under a high temperature of 500.degree.-1300.degree. C. and a high pressure of 1000-4000 kg/cm.sup.2, causes transition of pyrochlore phase into perovskite phase, thereby increasing the proportion of perovskite phase. Also treatment of a raw material represented by a general formula uPb(.sub.1/3 Nb.sub.2/3)O.sub.3 -vPbTiO.sub.3 (wherein u is an atomic ratio in a range of 0.5-1; and v is an atomic ratio in a range of 0.5- 0, with a relation u+v=1) and containing pyrochlore phase, under a high temperature of 500.degree.-1300.degree. C. and a high pressure of 1000-4000 kg/cm.sup.2 causes transition of pyrochlore phase into perovskite phase, thereby increasing the proportion of pervoskite phase.

REFERENCES:
patent: 4749668 (1988-06-01), Fujino et al.
patent: 4753905 (1988-06-01), Nishioka et al.
patent: 4959333 (1990-09-01), Mori et al.
Yonezawa et al., "The Crystal Structure and Piezoelectricity of the System Pb(Zn.sub.1/3 Nb.sub.2/3)O.sub.3 -PbTiO.sub.3 ", Jun. 3, 1969, Solid and Powder Metallurgy, vol. 16, No. 6, pp. 253-258.
Matsuo, Yoshihiro, "Synthesis of Perovskite-Type Complex Oxide Compound Pb(Zn.sub.1/3 Nb.sub.2/3)O.sub.3," 1970, pp. 46-58.

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