Method of manufacturing bis(cyclopentadienly)ruthenium and...

Organic compounds -- part of the class 532-570 series – Organic compounds – Heavy metal containing

Reexamination Certificate

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Reexamination Certificate

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07012150

ABSTRACT:
The present invention provides a method of manufacturing a bis(cyclopentadienyl)ruthenium, comprising the step of synthesizing a bis(cyclopentadienyl)ruthenium by causing cyclopentadiene, ruthenium chloride and zinc powder to react in an alcohol solvent, wherein the synthesis of the bis(cyclopentadienyl)ruthenium comprises the step of mixing the cyclopentadiene and zinc powder in the alcohol solvent and thereafter adding ruthenium chloride portionwise while holding the temperature of the reaction system at from −70° C. to 20° C. A highly pure product can be obtained through purification of subliming bis(cyclopentadienyl)ruthenium having been synthesized in the synthesis step in an atmosphere under reduced pressure.

REFERENCES:
patent: 5641871 (1997-06-01), Rohde et al.
patent: 6002036 (1999-12-01), Kadokura
patent: 2002/0161253 (2002-10-01), Voll et al.
Journal Chemical Society. Dalton, Vol'kenau et al., (1980), 1961-1964.
Journal of Organometallic Chemistry, Pertici et al., 288 (1985), 341-348.

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