Method of controlling a photoreaction with a laser beam

Chemistry: electrical and wave energy – Processes and products – Processes of treating materials by wave energy

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20415722, 20415741, 20415761, C07B 6100

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active

058082565

ABSTRACT:
A target is irradiated with a laser beam having an energy of h.nu.
, where n is an integer, instead of the photon energy h.nu. required for a reaction to proceed using a conventional single-photon excitation method. A desired reaction is selectively induced by the absorption of multiple photons instead of single photons. It is thus possible to induce a photoreaction in which an absorption is carried out in accordance with a selection theory different from that of single-photon absorption, and which is quite different from a photoreaction induced by a single-photon excitation. Namely, a target or reactant is irradiated with a photon energy h.nu..sub.2 having a wavelength integral times longer than that of the photon energy h.nu..sub.1 necessary for a photoreaction to proceed. Photon energy h.nu..sub.2 is either used in place of the photon energy h.nu..sub.1 necessary for a photoreaction, or together with the photon energy h.nu..sub.1, to thereby make the reactant absorb the energy equal to the photon energy h.nu..sub.1. The method is capable of selectively and preferentially inducing a specific photoreaction among various possible, concurrent photoreactions.

REFERENCES:
patent: 4350577 (1982-09-01), Heller
patent: 4461686 (1984-07-01), Tuccio et al.
patent: 4655890 (1987-04-01), Robinson et al.
"Two-Photon Photochromism of a Naphthopyran Derivative",M. Uchida and M. Irie, J. American Chemical Society, vol. 115, No. 14, 1993, 6442-6443.
"Detection and assignment of the `phantom` photochemical singlet of trans-stilbene by two-proton excitation", Stachelek et al., J. Chem. Phys., vol. 66, No. 10, 15 May 1977, 4541-4543.
Karlov N. K, "Laser Induced Chemical Reactions." Applied Optics. vol. 13, No. 2 Feb. 1974, 301-309.
"Detection and Assignment of the Phantom . . . " Stachelek et al, J. Chem. Phys, vol. 66, No. 10, 15 May 1977, 4541-4543.

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