Method for the production of 1-alkyl-6,7-methylene-dioxy-4(1H)-o

Organic compounds -- part of the class 532-570 series – Organic compounds – Four or more ring nitrogens in the bicyclo ring system

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549439, C07D491056, C07D31766

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active

044953518

ABSTRACT:
A method is disclosed for production of 1-alkyl-4(1H)-oxo-cinnolin-3-carboxylic acids. Mesoxalic acid dialkylester-3,4-methylenedioxy-phenylhydrazone is saponified using 1 to 1.5 Mol alkali into the corresponding monoalkylester, which is cyclicized with a Friedel-Crafts catalyst in the presence of a carboxylic acid anhydride into 6,7-methylenedioxy-4(1H)-oxo-cinnolin-3-carboxylic acid alkylester, which is alkylated with a C.sub.1 -C.sub.4 alkyl halogenide in the presence of alkali in a suitable solvent, after which the ester is saponified. Small amounts of byproduct alkylated in the 2-position are removed by brief heating and precipitation from alkaline solution, leaving a pure 1-alkyl product. The product is useful for the treatment of urinary tract infections.

REFERENCES:
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patent: 3669965 (1972-06-01), White
patent: 4264604 (1981-04-01), Sturm
Barber et al., J. Chem. Soc., 2828 (1961).
Ames et al., J. Chem. Soc., 5569 (1964).
Koga et al., J. Med. Chem., 23, 1358, (1980).

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