Method for the ionization of heavy molecules at atmospheric pres

Radiant energy – Ionic separation or analysis – With sample supply means

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250282, H01J 4910

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056635613

ABSTRACT:
The invention relates to a device and method for the ionization of non-vaporizable substance molecules at atmospheric pressure by chemical ionization (APCI=atmospheric pressure chemical ionization). The invention consists of desorbing the analyte substances which are mixed with decomposable substances (matrix substances) in solid form on a solid support, by laser irradiation at atmospheric pressure into a gas stream, and to add sufficient ions for proton transfer reactions to the gas stream. Explosives like cellulosis trinitrate or trinitro toluene (TNT) form a preferred class of decomposable matrix substances.

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Masahiko Tsuchiya et al., Liquid Ionization Mass Spectrometry of Nonvolatile Organic Compounds, Analytical Chemistry, vol. 56, pp. 14-19, Jan. 1984.
Ismet Dzidic et al., Atmospheric Pressure Ionization (API) Mass Spectrometry: Formation of Phenoxide Ions from Chlorinated Aromatic Compounds, Analytical Chemistry, vol. 47, pp. 1308-1312, Jul. 1975.
J. Yinon et al., An atmospheric pressure ionization (API) source for a magnetic sector mass spectrometer, Vacuum, vol. 26, pp. 159-161, Jan. 7, 1976.
Mattanjah S. de vries et al., Photoionization mass spectrometer with a microscope laser desorption source, Rev. Sci. Instrum., vol. 63, pp. 3321-3325, Jun. 1992.
Robert J. Cotter, Laser Desorption Chemical Ionization Mass Spectrometry, Analytical Chemistry, vol. 52, pp. 1767-1770, 1980.
R.E. Johnson, Models for matrix-assisted desorption by laser pulse, International Journal of Mass Spectrometry and Ion Processes, vol. 139, pp. 25-38, 1994.
Stephen G. Anderson et al., Determination of ion-ligand bond energies of ion fragmentation energies of electrospray-produced ions by collision-induced dissociation threshold measurements, vol. 141, pp. 217-219, Feb. 20, 1995.

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