Method for synthesizing N.sub.2 O.sub.5

Chemistry: electrical and wave energy – Processes and products – Electrostatic field or electrical discharge

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204103, C25B 100

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active

045252521

ABSTRACT:
A method and apparatus for electrochemically synthesizing N.sub.2 O.sub.5 includes oxidizing a solution of N.sub.2 O.sub.4 /HNO.sub.3 at an anode, while maintaining a controlled potential between the N.sub.2 O.sub.4 /HNO.sub.3 solution and the anode. A potential of about 1.35 to 2.0 V vs. SCE is preferred, while a potential of about 1.80 V vs. SCE is most preferred. Thereafter, the N.sub.2 O.sub.5 is reacted with either 1.5-diacetyl-3,7-dinitro-1,3,5,7-tetraazacyclooctane (DADN) or 1,3,5,7-tetraacetyl-1,3,5,7-tetraazacyclooctane (TAT) to form cyclotetramethylenetetraamine (HMX).

REFERENCES:
patent: 4443308 (1984-04-01), Coon et al.
J. Zawadski et al, "Electrochemical Preparation of Nitrogen Pentoxide", Rocznki Chemii, 22 (1948), 233.

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