Method for supporting metalloporphyrins on polybenzimidazole por

Catalyst – solid sorbent – or support therefor: product or process – Catalyst or precursor therefor – Organic compound containing

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502163, 502402, 521 53, 525417, 428 98, 428375, 428389, 428394, 428403, 428407, 428409, B01J 3106, C08J 936

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active

048001880

ABSTRACT:
A method for supporting metalloporphyrins on polybenzimidazole articles is disclosed herein. Microporous polybenzimidazole articles are treated with a strong base to produce an anionized polybenzimidazole article. A metalloporphyrin salt is dissolved in a solvent and is mixed with the anionized polybenzimidazole article to produce a microporous polybenzimidazole metalloporphyrin complex. This compound can be used in the selective oxidation of alkanes, olefins and aromatic compounds and is quite useful in the separation of oxygen from a gas stream. An alternative method of forming this complex by mixing directly the polybenzimidazole particulate with a weak metalloporphyrin salt without the use of a strong base results in lower percentages of substitution then does the principal method.

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Groves & Nemo: Aliphatic Hydroxylation Catalyzed by Iron Porphyrin Complexes: J. Am. Chem. S., vol. 105, pp. 6243-6248 (1983).
Tabushi & Morimitsu; Stereospecific; Regioselective & Catalytic Monoepoxidation, etc.; J. Amer. Chem. S., vol. 106, pp. 6871-6872, (1984).

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