Method for selectively reducing plutonium values by a photochemi

Chemistry: electrical and wave energy – Processes and products – Processes of treating materials by wave energy

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423 10, 423251, C01G 5600, B01J 110

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active

041315278

ABSTRACT:
The rate of reduction of Pu(IV) to Pu(III) in nitric acid solution containing a reducing agent is enhanced by exposing the solution to 200-500 nm electromagnetic radiation. Pu values are recovered from an organic extractant solution containing Pu(IV) values and U(VI) values by the method of contacting the extractant solution with an aqueous nitric acid solution in the presence of a reducing agent and exposing the aqueous solution to electromagnetic radiation having a wavelength of 200-500 nm. Under these conditions, Pu values preferentially distribute to the aqueous phase and U values preferentially distribute to the organic phase.

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patent: 4080273 (1978-03-01), De Poorter et al.
Streeton et al., "The Preparation, Stabilisation and Analysis of Uranium (IV) Nitrate Solutions," UKAEA Report, AERE R- 3938, 1962.
Wick, "Plutonium Handbook," vol. II, p. 523, Gordon & Breach, (1967), New York.
Horner et al., "Laboratory Development of Solvent Extraction Processes for Spent LMFBR Fuels," ORNL/TM-5729, pp. 74, 75 & 90, Jan. 1977.
Bell et al., J. Inorg. Nucl. Chem., 38, 831-835, (1976).

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