Method for removal of MW176 cyclic acetal formed during the...

Organic compounds -- part of the class 532-570 series – Organic compounds – Oxygen containing

Reexamination Certificate

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C568S852000, C568S861000, C568S868000, C568S872000

Reexamination Certificate

active

06969779

ABSTRACT:
The present invention is an improvement upon the process for the production of 1,3-propanediol (PDO) wherein an aqueous solution of 3-hydroxypropanal (HPA) is formed, and the HPA is subjected to hydrogenation to produce a crude PDO mixture comprising PDO, water, MW176 acetal, and high and low volatility materials, wherein the crude PDO mixture is dried to produce a first overhead stream comprising water and some high volatility materials and a dried crude PDO mixture as a first distillate bottoms stream comprising PDO, MW176 acetal, and low volatility materials, and wherein the dried crude PDO mixture is distilled to produce a second overhead stream comprising some high volatility materials, a middle stream comprising PDO and MW176 acetal, and a second distillate bottoms stream comprising PDO and low volatility materials. The improvement on this process comprises treating the crude PDO mixture and/or the dried crude PDO mixture and/or the PDO product with an acidic zeolite, an acid form cation exchange resin, or a soluble acid to convert the MW176 cyclic acetal to more volatile materials which can be easily separated from PDO by distillation.

REFERENCES:
patent: 5008473 (1991-04-01), Breitkopf et al.
patent: 5527973 (1996-06-01), Kelsey
patent: 5786524 (1998-07-01), Powell et al.
patent: 6235948 (2001-05-01), Sunkara et al.
patent: 0983985 (2000-03-01), None
patent: WO 98/49216 (1998-11-01), None
patent: WO 00/10953 (2000-03-01), None
patent: WO 00/14041 (2000-03-01), None

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