Method for preparing diaryl carbonates with improved selectivity

Organic compounds -- part of the class 532-570 series – Organic compounds – Carbonate esters

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558271, 558272, 558273, C07C 6800

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059170778

ABSTRACT:
Diaryl carbonates such as diphenyl carbonate are prepared by reaction of hydroxyaromatic compounds such as phenol with oxygen and carbon monoxide in the presence of a catalyst composition comprising a Group VIIIB metal such as palladium or a compound thereof, a bromide source such as a quaternary ammonium or hexaalkylguanidinium bromide and a polyaniline in partially oxidized and partially reduced form. The polyaniline is preferably halide-doped and in the form of a blend with a binder polymer containing ether or ester groups and a complex-forming salt.

REFERENCES:
patent: 5231210 (1993-07-01), Joyce et al.
patent: 5284964 (1994-02-01), Pressman et al.
patent: 5312955 (1994-05-01), Pressman
patent: 5399734 (1995-03-01), King, Jr. et al.
U.S. Patent Application Serial No. 08/929,000, filed Sep. 13, 1997, by Eric J. Pressman et al., entitled "Method for Preparing Diaryl Carbonates Employing Hexaalkylguanidinium Halides".
U.S. Patent Application Serial No. 09/040,264, filed Aug. 27, 1997, by Eric J. Pressman et al., entitled "Method for Preparing Diaryl Carbonates Employing Hexaalkylguanidinium Halides".

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