Method for preparing crystalline aluminosilicates

Chemistry of inorganic compounds – Silicon or compound thereof – Oxygen containing

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252455Z, 260448C, 423328, C01B 3328

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043761046

ABSTRACT:
Crystalline aluminosilicates having a high silica to alumina molar ratio are prepared by mixing a source of silica, a source of alumina, a source of alkali metal, water and one or more substituted neopentylamines having the formula: ##STR1## wherein R.sup.2 is H, OH or NH.sub.2 and R.sup.1 is a C.sub.1 to C.sub.6 alkyl group, and maintaining the mixture under conditions of elevated temperature and pressure, typically in the range from 80.degree. to 210.degree. C. and autogenous pressure for a time sufficient to effect formation of the aluminosilicate, typically not less than 4 hours. The molar ratio of silica to alumina in the initial mixture is suitably in the range from 10:1 to 150:1 and the amounts of alkali metal and neopentylamine are suitably in the range from 2:1 to 0.02:1 and 10:1 to 0.02:1 respectively moles per mole equivalent of total silica and alumina in the respective sources. Depending on the ratio of silica to alumina in the initial mixture crystalline aluminosilicates having a mordenite structure or a ZSM-5 type zeolite structure or mixtures thereof may be prepared. Mordenites having a silica to alumina ratio greater than 10:1 can be prepared.

REFERENCES:
patent: 3506400 (1970-04-01), Eberly et al.
patent: 4107195 (1978-08-01), Rollmann
patent: 4151189 (1979-04-01), Rubin et al.
patent: 4242233 (1980-12-01), Ball
Voorhies "J. of Catalysis" 22, 1971, 419-426.

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